Don’t like how Photobooth gives you that white flash or counts down from three to take a picture? Hold the Shift key down when you press the picture button and it will stop the flash. Hold down the Option key and the picture will take immediately. You can hold down both if you like as well.
Related: Photobooth locked in Pages, Create A Screen Shot, Windows Resizing Options, Shortcuts For System Preferences, Screen Capture a Window.
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