MacMost Q&A Forum • View All Forum Questions • Ask a Question 7/16/105:13 pm Delete a photo library on the iPhone How do you delete a photo libray from iphone? — veronica sobrevilla Comments: One Response to “Delete a photo library on the iPhone” Gary Rosenzweig 9 years ago Those albums are synced from iPhoto. So connect your iPhone, and then use iTunes to change your sync settings so that album does not sync to your iPhone. Then sync again to apply the changes. Comments Closed.