MacMost Q&A Forum • View All Forum Questions • Ask a Question 7/16/105:13 pm Delete a photo library on the iPhone How do you delete a photo libray from iphone? — veronica sobrevilla Comments: One Response to “Delete a photo library on the iPhone” Gary Rosenzweig 10 years ago Those albums are synced from iPhoto. So connect your iPhone, and then use iTunes to change your sync settings so that album does not sync to your iPhone. Then sync again to apply the changes. Related Video Tutorials: Search Your Photo Library For Objects ― How To Optimize Photo Storage On Your iPhone ― Managing a Video Library On Your Mac Comments Closed.